Released on Marianne Faithfull's 2008 compilation album, 'As Tears Go By' stands as a defining track from her early career, originally recorded in 1964. The song features a haunting, minimalist arrangement that highlights Faithfull's distinctive vocal delivery and the era's emerging folk-rock aesthetic. As one of her most recognizable compositions, it captures a mood of introspective melancholy that became central to her public image during the mid-1960s. The recording exemplifies the raw emotional honesty characteristic of her work, influencing subsequent generations of artists who sought to blend personal narrative with atmospheric soundscapes. Its enduring popularity ensures its place as a staple in discussions of classic British music and the evolution of the singer-songwriter genre.